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Article

Reversible disorder-order transitions in atomic crystal nucleation
Author Jeon, Sungho; Heo, Taeyeong; Hwang, Sang-Yeon; Ciston, Jim; Bustillo, Karen C.; Reed, Bryan W.; Ham, Jimin; Kang, Sungsu; Kim, Sungin; Lim, Joowon; Lim, Kitaek; Kim, Ji Soo; Kang, Min-Ho; Bloom, Ruth S.; Hong, Sukjoon; Kim, Kwanpyo; Zettl, Alex; Kim, Woo
Corresponding Author Info Prof. Lee, Won Chul (기계공학과)
Professor
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E-mail 메일wonchullee@hanyang.ac.kr
Document Type
바카라 토토 Science2021, 371, 6528, 498
Times 바카라 토토 21 (2022.2.21.)
External Information
Abstract
[History]
- 2021년 July/August부로, 이 highly 바카라 토토 paper 의 인용 횟수가 분야와 출판 연도에 대해 인용 빈도가 높은 임계값을 기반으로 Chemistry 학술 분야에서 상위 1%에 올랐습니다.

[Abstract]
Nucleation in atomic crystallization remains poorly understood, despite advances in classical nucleation theory. The nucleation process has been described to involve a nonclassical mechanism that includes a spontaneous transition from disordered to crystalline states, but a detailed understanding of dynamics requires further investigation. In situ electron microscopy of heterogeneous nucleation of individual gold nanocrystals with millisecond temporal resolution shows that the early stage of atomic crystallization proceeds through dynamic structural fluctuations between disordered and crystalline states, rather than through a single irreversible transition. Our experimental and theoretical analyses support the idea that structural fluctuations originate from size-dependent thermodynamic stability of the two states in atomic dusters. These findings, based on dynamics in a real atomic system, reshape and improve our understanding of nucleation mechanisms in atomic crystallization.
Web of Science Categories Multidisciplinary Sciences
Funding
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